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Enzyme-catalysed acylation as a new strategy for oligosaccharide synthesis with minimal protection

ReferenceE11765
Principal Investigator / Supervisor Professor Benjamin Davis
Co-Investigators /
Co-Supervisors
Professor Antony Fairbanks
Institution University of Oxford
DepartmentDyson Perrins Laboratory
Funding typeResearch
Value (£) 176,163
StatusCompleted
TypeResearch Grant
Start date 24/01/2000
End date 24/04/2002
Duration27 months

Abstract

There still exists no generally applicable method for the efficient and stereoselective formation of glycosidic bonds. Whilst the tethering of glycosyl acceptors to glycosyl donors allows the formation of glycosidic bonds with a higher degree of stereocontrol, present approaches are hampered by laborious protection regimes. An approach to the tethering of unprotected donors and acceptors through the enzyme-catalysed regioselective formation of esters and mixed disulphide links is described. Suitable activation should allow the formation of glycosidic bonds, in a manner that readily lends itself to facile iteration. It is proposed that variations in the nature and length of the introduced tether will determine the stereochemistry of the newly formed anomeric centre.

Summary

unavailable
Committee Closed Committee - Engineering & Biological Systems (EBS)
Research TopicsX – not assigned to a current Research Topic
Research PriorityX – Research Priority information not available
Research Initiative X - not in an Initiative
Funding SchemeX – not Funded via a specific Funding Scheme
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