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Mechanistic mapping and redox regulation in NO- synthase and a related monooxygenase

ReferenceC10203
Principal Investigator / Supervisor Professor Stephen Chapman
Co-Investigators /
Co-Supervisors
Institution University of Edinburgh
DepartmentSch of Chemistry
Funding typeResearch
Value (£) 182,153
StatusCompleted
TypeResearch Grant
Start date 01/10/1998
End date 31/12/2001
Duration38 months

Abstract

The nitric oxide synthases are eukaryotic P450-like flavocytochromes which catalyse the production of citrulline and nitric oxide (NO) from arginine. They are important enzymes because of the roles of NO in cellular signalling processes. We aim to investigate the way in which the redox properties of neuronal nitric oxide synthase (nNOS) are regulated. This will be achieved by determining the underlying thermodynamic and kinetic properties of the enzyme. In addition we shall exploit the similarities between nNOS and its closest prokaryotic relative, flavocytochrome P450 BM3 to further examine the distinct mechanisms by which electron transfer is controlled. This will be done using chimeras between nNOS and P450 BM designed to switch the redox control mechanisms in these enzymes.

Summary

unavailable
Committee Closed Committee - Biochemistry & Cell Biology (BCB)
Research TopicsX – not assigned to a current Research Topic
Research PriorityX – Research Priority information not available
Research Initiative X - not in an Initiative
Funding SchemeX – not Funded via a specific Funding Scheme
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