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The structure and mechanism of catalysis of the photosynthetic water oxidising complex

ReferenceC09203
Principal Investigator / Supervisor Professor J Nugent
Co-Investigators /
Co-Supervisors
Professor M Evans
Institution University College London
DepartmentGenetics Evolution and Environment
Funding typeResearch
Value (£) 185,750
StatusCompleted
TypeResearch Grant
Start date 03/09/1998
End date 31/10/2001
Duration38 months

Abstract

Water oxidation by photosystem II of plants, algae and cyanobacteria is the source of reductant for the biosphere and oxygen in the atmosphere. Water oxidation is catalysed by a Mn complex which accumulates oxidising equivalents following the single electron turnover of photosystem II. The detailed structure and mechanism of catalysis of water oxidation by the complex is unknown. Recent work in our laboratory has identified methods for stabilisation and detection by EPR spectroscopy of previously inaccessible redox states of the Mn complex. A programme is proposed using magnetic resonance and X-ray spectroscopy which will determine the characteristics of substrate binding to the Mn complex and definitively identify the oxidation state of Mn during turnover of the complex. A robust model of the catalytic process will be defined.

Summary

unavailable
Committee Closed Committee - Biochemistry & Cell Biology (BCB)
Research TopicsX – not assigned to a current Research Topic
Research PriorityX – Research Priority information not available
Research Initiative X - not in an Initiative
Funding SchemeX – not Funded via a specific Funding Scheme
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