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New methods and strategies for oligosaccharide assembly

ReferenceBCI06178
Principal Investigator / Supervisor Professor Steven Ley
Co-Investigators /
Co-Supervisors
Institution University of Cambridge
DepartmentChemistry
Funding typeResearch
Value (£) 280,750
StatusCompleted
TypeResearch Grant
Start date 01/09/1996
End date 01/01/2000
Duration40 months

Abstract

To investigate new protecting groups and novel reactivity control strategies for the synthesis of complex oligosaccharide arrays. We have developed the CyclohexaneDiAcetal group which shows good selectivity for transdiequatorial 1,2 diols.We will prepare chiral CDA protecting groups, which we expect to show enhanced selectivity in protection reactions where there are two pairs of diols and take part in desymmetrisation using the principles of chirality matching and mis-matching. We will also investigate new deprotection strategies. Our goal is to develop CDA protecting groups that may be removed using a variety of different reagent systems. We will combine our multiple sequential glycosidation strategy using reactivity tuning of the glycoside donors with orthogonal glycosidation to allow large saccharide blocks to be assembled quickly and efficiently.

Summary

unavailable
Committee Closed Committee - Biomolecular Sciences (BMS)
Research TopicsX – not assigned to a current Research Topic
Research PriorityX – Research Priority information not available
Research Initiative Biological Chemistry Initiative (BCI) [1995]
Funding SchemeX – not Funded via a specific Funding Scheme
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