Award details

Chemical mechanism and 3-D active site of methylaspartate ammonia-lyase

ReferenceBCI05857
Principal Investigator / Supervisor Professor David Gani
Co-Investigators /
Co-Supervisors
Institution University of Birmingham
DepartmentSchool of Chemistry
Funding typeResearch
Value (£) 149,663
StatusCompleted
TypeResearch Grant
Start date 01/12/1996
End date 01/02/2000
Duration38 months

Abstract

Previous work on methylaspartase in our own laboratory and work on partially homologous enzymes in others' laboratories has reached the stage where a full 3-D mechanistic picture of the methylaspartase reaction is timely and feasible. The current application seeks to draw previous kinetic, kinetic isotope, substrate specificity, SAR, chemical model and amino acid sequence data into a 3-D context using the fact that the metal ion binding regions of methylaspartase are similar to more simple enzymes. The scientific objectives are to completely characterise a dehydroalanine residue and determine the exact role of the metal ions. Chemical synthesis, physical organic chemistry, site-directed mutagenesis and NMR will play major roles in these studies.

Summary

unavailable
Committee Closed Committee - Biomolecular Sciences (BMS)
Research TopicsX – not assigned to a current Research Topic
Research PriorityX – Research Priority information not available
Research Initiative Biological Chemistry Initiative (BCI) [1995]
Funding SchemeX – not Funded via a specific Funding Scheme
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